Hidden Bibliographic Details
ISBN: | 9783319605319 3319605313 3319605305 9783319605302 9783319605302
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Digital file characteristics: | text file PDF
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Notes: | "Doctoral thesis accepted by University of Stuttgart, Germany." Includes bibliographical references. Online resource; title from PDF title page (SpringerLink, viewed July 11, 2017).
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Summary: | This thesis presents an experimental study of ordering phenomena in rare-earth nickelate-based heterostructures by means of inelastic Raman light scattering and elastic resonant x-ray scattering (RXS). Further, it demonstrates that the amplitude ratio of magnetic moments at neighboring nickel sites can be accurately determined by RXS in combination with a correlated double cluster model, and controlled experimentally through structural pinning of the oxygen positions in the crystal lattice. The two key outcomes of the thesis are: (a) demonstratingfull control over the charge/bond and spin order parameters in specifically designed praseodymium nickelate heterostructures and observation of a novel spin density wave phase in absence of the charge/bond order parameter, which confirms theoretical predictions of a spin density wave phase driven by spatial confinement of the conduction electrons; and (b) assessing the thickness-induced crossover between collinear and non-collinear spin structures in neodymium nickelate slabs, which is correctly predicted by drawing on density functional theory.
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Other form: | Printed edition: 9783319605302
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Standard no.: | 10.1007/978-3-319-60531-9
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